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Assuming you installed LO without error messages, you have 2 option to assign CALC to the 2 extensions.

1) Right-click on a .csv/.xls file in windows explorer, select Open With.. In the window that pops up, you should see CALC ( as SCALC.EXE) or browse for it. C:\program files(x86)\Libreoffice3.6\Program. There is a tiny check box at the bottom of this window "Always use this program to open this file type" that needs to be checked. Click OK.

2) Control Panel -> Default Programs and Associate a file type or protocol with a program.