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The only way to obtain arbitrary fractions is to use a font with the OpenType table "frac". For example, with Libertinus Serif you need to use as font name

Libertinus Serif:frac

to obtain

image description

You need to create a character style to use for your fractions. Note that not all fonts support OpenType features, so check the capabilities of your font first.

For more information about OpenType and LibreOffice see my article on OpenSource.com site or stay tuned to my personal blog ;)